The Chad Pennington Marshall teams - the MAC was pretty freaking great from about 1997-05. They had IMO the best conf championship games, December weather, home game CCGs, rivalaries, etc. Why did Marshall ever leave this conference for away games at Rice?
Bit of history during Marshall's undefeated season they were 11-0 going into the game w/ WMU (ranked #12). They got spanked and were down 23-0 in the 3rd quarter and mounted a furious comeback to win 34-30 on a last sec TD. If they would have lost they wouldn't have gone to a bowl game.
PSU 1994 - I guess there have been better offenses if you go by yardage and PPG, especially today. But they played the most asthetically beautiful offense that I have ever seen.
Arizona last year - RIP Khail Tate.
Alabama - the Paul Palmer years. Bama was much more lovable when they'd go 9-3 or 10-2 and had their cute little QB/RB/WR hybrids
As far as Major Harris goes, I think he was better than Vick. Unfortunately in Major's final year, WVU had one of the worst OLs in D1 (it was almost PSU in the Hackenberg years bad) and spent the entire season running for his life.